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• W2335441010 startingPage "9524" @default.
• W2335441010 abstract "An FeV(O) complex has been synthesized from equimolar solutions of (Et4N)2[FeIII(Cl)(biuret-amide)] and mCPBA in CH3CN at room temperature. The FeV(O) complex has been characterized by UV–vis, EPR, Mössbauer, and HRMS and shown to be capable of oxidizing a series of alkanes having C–H bond dissociation energies ranging from 99.3 kcal mol–1 (cyclohexane) to 84.5 kcal mol–1 (cumene). Linearity in the Bell–Evans–Polayni graph and the finding of a large kinetic isotope effect suggest that hydrogen abstraction is engaged the rate-determining step." @default.
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• W2335441010 date "2014-01-16" @default.
• W2335441010 modified "2023-10-11" @default.
• W2335441010 title "Formation of a Room Temperature Stable Fe^V(O) Complex: Reactivity Toward Unactivated C–H Bonds" @default.
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• W2335441010 doi "https://doi.org/10.1021/ja412537m" @default.
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