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- W2335500056 abstract "By taking advantage of vinyl aziridines as a heteroatom-containing five-atom component in rhodium-catalyzed intramolecular formal hetero-[5 + 2] cycloaddition reactions with alkynes, a highly efficient method for the synthesis of fused azepine derivatives at 30 °C was developed. The reaction has broad substrate scope and tolerates a wide range of functional groups. The chirality of vinyl aziridine-alkyne substrates can be completely transferred to the cycloadducts, representing an atom-economic and enantiospecific protocol for the construction of fused 2,5-dihydroazepines for the first time." @default.
- W2335500056 created "2016-06-24" @default.
- W2335500056 creator A5043291054 @default.
- W2335500056 creator A5046202330 @default.
- W2335500056 creator A5048609660 @default.
- W2335500056 creator A5084000645 @default.
- W2335500056 date "2015-03-16" @default.
- W2335500056 modified "2023-10-10" @default.
- W2335500056 title "Transfer of Chirality in the Rhodium-Catalyzed Intramolecular Formal Hetero-[5 + 2] Cycloaddition of Vinyl Aziridines and Alkynes: Stereoselective Synthesis of Fused Azepine Derivatives" @default.
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- W2335500056 doi "https://doi.org/10.1021/jacs.5b01305" @default.
- W2335500056 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25763476" @default.
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