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• W2335596671 abstract "Chalcogenide glasses with tetrahedral networks can undergo significant densification under pressure owing to their open structures. The structural mechanisms of pressure-induced densification and the corresponding evolution of physical properties of glassy GeSe4 alloy are studied over pressures ranging between ambient and 32.5 GPa, using X-ray scattering supplemented with 3D Monte Carlo structural modeling, Raman spectroscopy, electrical conductivity, and P–V equation of state measurements. The results demonstrate a pressure-induced, hysteretically reversible transition between low-density semiconducting and high-density metallic amorphous phases of GeSe4 near ∼10–15 GPa. These two phases are characterized by their distinct P–V equations of state and structural mechanisms of densification. Densification in the low-density phase is dominated by large inward shifting of the second neighbors with a small amount of conversion from edge-sharing to corner-sharing GeSe4 tetrahedra. On the other hand, densificati..." @default.
• W2335596671 created "2016-06-24" @default.
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• W2335596671 date "2014-03-04" @default.
• W2335596671 modified "2023-09-23" @default.
• W2335596671 title "Polyamorphism and Pressure-Induced Metallization at the Rigidity Percolation Threshold in Densified GeSe₄ Glass" @default.
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• W2335596671 doi "https://doi.org/10.1021/jp4108602" @default.
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