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• W2335676993 startingPage "10260" @default.
• W2335676993 abstract "Morphology-controlled synthesis of tantalates is a major challenge in the field of material science. Herein, an innovative strategy has been developed for controllably synthesizing K1.9Na0.1Ta2O6·2H2O (KNTO) nanocrystals shaped as octahedra and nanosheets without using any capping agents. The obtained nanocrystals show high activity in photocatalytic H2 evolution from CH3OH/H2O solution, and their performance closely depends on the exposed facets, in which the {111}-facet-bounded nanooctahedra exhibit more than 3 times higher activity than the nanosheets dominated with {101} facets. The influence of surface atomic structure and electronic band structure on the photocatalytic properties of the KNTO nanocrystals is systematically studied. This is the first report for the facet controllable synthesis of tantalate materials with highly regular shapes. The present approach is anticipated as a general strategy for controllable synthesis of tantalate materials and also provides feasibility for rational design and activity optimization of shape-controlled photocatalysts for H2 production." @default.
• W2335676993 created "2016-06-24" @default.
• W2335676993 creator A5000249135 @default.
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• W2335676993 date "2013-10-09" @default.
• W2335676993 modified "2023-09-28" @default.
• W2335676993 title "Tuning Activities of K_1.9Na_0.1Ta₂O₆<i>·</i>2H₂O Nanocrystals in Photocatalysis by Controlling Exposed Facets" @default.
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• W2335676993 doi "https://doi.org/10.1021/am403025q" @default.
• W2335676993 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24025326" @default.
• W2335676993 hasPublicationYear "2013" @default.
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