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- W2335898678 abstract "The intramolecular Diels-Alder reaction has been used as a powerful method to access the tricyclic core of the eunicellin natural products from a number of 9-membered-ring precursors. The endo/exo selectivity of this reaction can be controlled through a remarkable organocatalytic approach, employing MacMillan's imidazolidinone catalysts, although the mechanistic origin of this selectivity remains unclear. We present a combined experimental and density functional theory investigation, providing insight into the effects of medium-ring constraints on the organocatalyzed intramolecular Diels-Alder reaction to form the isobenzofuran core of the eunicellins." @default.
- W2335898678 created "2016-06-24" @default.
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- W2335898678 date "2015-11-30" @default.
- W2335898678 modified "2023-10-14" @default.
- W2335898678 title "Medium-Ring Effects on the <i>Endo/Exo</i> Selectivity of the Organocatalytic Intramolecular Diels–Alder Reaction" @default.
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- W2335898678 doi "https://doi.org/10.1021/acs.joc.5b02037" @default.
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