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- W2336697034 abstract "Artificial photosynthesis by photoelectrocatalytic CO2 reduction is dependent, as is natural photosynthesis, on interfacial electron transfer to couple light excitation energy to reaction centers. For heterogeneous systems, in the context of frontier orbital theory artificial reaction centers are defined through the interactions of filled and empty orbitals within a few electronvolts of the Fermi energy of the adsorbate complex. Here we report a scanning tunneling microscopy (STM) and density functional theory investigation of the orbital-resolved adsorption state defining the dative bonding interaction between a III–V semiconductor surface [GaP(110)] and a N-containing heteroaromatic (pyridine). This system was selected for its relevance to photoelectrocatalysis utilizing heteroaromatic cocatalysts, which has been reported to yield highly selective CO2 reduction to fuels. By examining the distribution of unoccupied molecular orbitals, we show that STM images can be used to positively identify the sites o..." @default.
- W2336697034 created "2016-06-24" @default.
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- W2336697034 date "2015-12-17" @default.
- W2336697034 modified "2023-10-18" @default.
- W2336697034 title "Orbital-Resolved Imaging of the Adsorbed State of Pyridine on GaP(110) Identifies Sites Susceptible to Nucleophilic Attack" @default.
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- W2336697034 doi "https://doi.org/10.1021/acs.jpcc.5b08659" @default.
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