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• W2339118665 abstract "Motivated by recent Mossbauer experiments on strongly correlated mixed-valence systems, we revisit the Kubo-Anderson stochastic theory of spectral lineshapes. Using a Majorana representation for the nuclear spin we demonstrate how to recast the classic lineshape theory in a field-theoretic and diagrammatic language. We show that the leading contribution to the self-energy can reproduce most of the observed lineshape features including splitting and lineshape narrowing, while the vertex and the self-consistency corrections can be systematically included in the calculation. This new approach permits us to predict the line-shape produced by an arbitrary bulk charge fluctuation spectrum providing a model-independent way to extract the local charge fluctuation spectrum of the surrounding medium. We also derive an inverse formula to extract the charge fluctuation from the measured lineshape." @default.
• W2339118665 created "2016-06-24" @default.
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• W2339118665 date "2016-08-08" @default.
• W2339118665 modified "2023-09-27" @default.
• W2339118665 title "Majorana approach to the stochastic theory of line shapes" @default.
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• W2339118665 doi "https://doi.org/10.1103/physrevb.94.085113" @default.
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