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• W2340772117 abstract "We report our investigation of the electronic and magnetic excitations of ${mathrm{Sr}}_{3}{mathrm{NiIrO}}_{6}$ by resonant inelastic x-ray scattering at the Ir ${L}_{3}$ edge. The intra-${t}_{2g}$ electronic transitions are analyzed using an atomic model, including spin-orbit coupling and trigonal distortion of the ${mathrm{IrO}}_{6}$ octahedron, confronted with ab initio quantum chemistry calculations. The Ir spin-orbital entanglement is quantified and its implications for the magnetic properties, in particular in inducing highly anisotropic magnetic interactions, are highlighted. These are included in the spin-wave model proposed to account for the dispersionless magnetic excitation that we observe at $90phantom{rule{0.28em}{0ex}}mathrm{m}mathrm{e}mathrm{V}$. By counterbalancing the strong ${mathrm{Ni}}^{2+}$ easy-plane anisotropy that manifests itself at high temperature, the anisotropy of the interactions finally leads to the remarkable easy-axis magnetism reported in this material at low temperature." @default.
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• W2340772117 date "2016-06-01" @default.
• W2340772117 modified "2023-10-16" @default.
• W2340772117 title "Anisotropic interactions opposing magnetocrystalline anisotropy in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mi>NiIrO</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W2340772117 doi "https://doi.org/10.1103/physrevb.93.224401" @default.
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