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- W2341866883 abstract "Graphitic carbon nitride (CN) is an emerging photocatalyst with promising prospect, but presently it still falls short on photocatalytic efficiency and photoresponsive range. We herein constructed a novel ternary heterostructure by hybridization of conducting polymer and semiconductor with CN. The exfoliated two dimension CN nanosheets (CN-NSs) are superior to bulk CN as both catalysts and supporting materials. Most recently, there are few reports involving the construction of heterojunction photocatalysts using CN-NSs as supports. The improvement of charge separation efficiency, specific surface area and visible light harvesting is simultaneously achieved in such a novel ternary heterostructure due to the synergetic effect of polyaniline (PANI) and ZnO coupling. As a result, the CN-NS/PANI/ZnO photocatalyst possesses excellent visible photocatalytic performance for MB and 4-CP degradation with a rate constant of 0.026 and 0.0049min(-1), which is about 3.6 and 3.3 times of CN, respectively. The enhanced mechanism is proposed based on the confirmation of OH and h(+) as main oxidative species. Overall, this work can not only yield high-efficient visible photocatalysts but also provide deeper insight into the enhanced mechanisms of CN-NS-based ternary heterostructure." @default.
- W2341866883 created "2016-06-24" @default.
- W2341866883 creator A5038040931 @default.
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- W2341866883 date "2016-08-01" @default.
- W2341866883 modified "2023-10-16" @default.
- W2341866883 title "Constructing a novel carbon nitride/polyaniline/ZnO ternary heterostructure with enhanced photocatalytic performance using exfoliated carbon nitride nanosheets as supports" @default.
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- W2341866883 doi "https://doi.org/10.1016/j.jhazmat.2016.04.035" @default.
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