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- W2342419412 abstract "A three-dimensional geometry model of the particle/monolithic two-stage reactor with beds-interspace distributed dioxygen feeding for oxidative coupling of methane (OCM) was set up. The improved Stansch kinetic model adapting different operating temperatures was established to calculate the OCM reactor performance using computational fluid dynamics (CFD) and FLUENT software. The results showed that the calculated values matched well with the experimental values of the conversion of CH4 and the selectivity of products (C2H6, C2H4, CO2, CO) in the OCM reactor. The distributed dioxygen feeding with the percentage of 5–20% based oxygen flow rate of top inlet promoted the OCM reaction in monolithic catalyst bed and led to the conversion of CH4 and the selectivity and yield of C2 (C2H6 and C2H4) increase obviously. The distributed dioxygen feeding was 15%, the conversion of CH4, the selectivity and the yield of C2 reached 34.1%, 68.2% and 23.3%, respectively." @default.
- W2342419412 created "2016-06-24" @default.
- W2342419412 creator A5013707926 @default.
- W2342419412 creator A5025757361 @default.
- W2342419412 date "2016-07-01" @default.
- W2342419412 modified "2023-10-17" @default.
- W2342419412 title "Numerical simulation of particle/monolithic two-stage catalyst bed reactor with beds-interspace distributed dioxygen feeding for oxidative coupling of methane" @default.
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- W2342419412 doi "https://doi.org/10.1016/j.compchemeng.2016.04.036" @default.
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