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- W2342838352 abstract "Photocatalytic hydrogen (H 2 ) evolution requires efficient electron transfer to catalytically active sites in competition with charge recombination. Thus, controlling charge‐carrier dynamics in the photocatalytic H 2 evolution process is essential for optimized photocatalyst nanostructures. Here, the efficient delocalization of electrons is demonstrated in a heterostructure consisting of optimized MoS 2 tips and CdS nanorods (M‐t‐CdS Nrs) synthesized by amine‐assisted oriented attachment. The heterostructure achieves photocatalytic H 2 activity of 8.44 mmol h −1 g −1 with excellent long‐term durability (>23 h) without additional passivation under simulated solar light (AM 1.5, 100 mW cm −2 ). This activity is nearly two orders of magnitude higher than that of pure CdS Nrs. The impressive photocatalytic H 2 activity of M‐t‐CdS Nrs reflects favorable charge‐carrier dynamics, as determined by steady‐state PL and time‐correlated single photon counting correlation analysis at low temperature. The MoS 2 cocatalysts precisely located at the end of the CdS Nrs exhibit ultrafast charge transfer and slow charge recombination via spatially localized deeper energy states, resulting in a highly efficient H 2 evolution reaction in lactic acid containing an electrolyte." @default.
- W2342838352 created "2016-06-24" @default.
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- W2342838352 date "2016-04-25" @default.
- W2342838352 modified "2023-10-17" @default.
- W2342838352 title "Delocalized Electron Accumulation at Nanorod Tips: Origin of Efficient H<sub>2</sub> Generation" @default.
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- W2342838352 doi "https://doi.org/10.1002/adfm.201600285" @default.
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