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• W2343463178 endingPage "1311" @default.
• W2343463178 startingPage "1304" @default.
• W2343463178 abstract "In this work, molecular-symmetry enhanced 13CO natural abundant isotopic infrared transition was identified in Mn(CO)5Br dissolved in CCl4 by FTIR spectroscopy. Diagonal and associated off-diagonal two-dimensional IR (2D IR) peaks of the 13CO-species were found to be spectrally separated from the all-12CO species, allowing a direct probe of the 13C natural abundant ensemble. Temperature-dependent FTIR experiment showed no evidence of ligand exchange in the metal carbonyl complex. Intramolecular vibrational redistribution dynamics among the CO stretching vibrational states were extracted using population-time dependent 2D IR diagonal and off-diagonal peaks for both radial mono-13CO and all-12CO isotopomers. This work demonstrates the potential use of natural abundant isotopic molecular species as a probe for revealing equilibrium and nonequilibrium structural dynamics in condensed-phase molecular systems." @default.
• W2343463178 created "2016-06-24" @default.
• W2343463178 creator A5010954184 @default.
• W2343463178 creator A5052272042 @default.
• W2343463178 creator A5085432519 @default.
• W2343463178 date "2016-02-17" @default.
• W2343463178 modified "2023-10-16" @default.
• W2343463178 title "Two-Dimensional Infrared Study of 13C-Natural Abundant Vibrational Transition Reveals Intramolecular Vibrational Redistribution Rather than Fluxional Exchange in Mn(CO)5Br" @default.
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• W2343463178 doi "https://doi.org/10.1021/acs.jpcb.5b11310" @default.
• W2343463178 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26836759" @default.
• W2343463178 hasPublicationYear "2016" @default.
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