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- W2344618650 abstract "Abstract Mixed matrix membranes (MMMs) were composed of imidazole functionalized graphene oxide (ImGO), a CO 2 -philic nano-sheet inorganic material, and poly(ether- b -amide) (PEBAX) for CO 2 capture. MMM doped with 0.8 wt.% ImGO exhibits the best CO 2 separation performance, which shows the CO 2 /N 2 selectivity up to 105.5 combined with CO 2 permeability of 76.2 Barrer (1 Barrer = 10 −10 cm 3 (STP) cm cm −2 s −1 cmHg −1 ), surpassing the Robeson Upper Bound of 2008. The selectivity of MMM for CO 2 /N 2 increases by 46.0% compared to the Pristine PEBAX due to the interaction between CO 2 and imidazole groups. With the increase of feed pressure, CO 2 permeability increases significantly because of its higher solubility in polymer matrix and plasticization. It is effective to separation CO 2 from N 2 at lower temperature for MMMs because the apparent activation energy of the N 2 permeation process in ImGO/PEBAX MMMs is much higher than that of CO 2 . Tg of MMMs are increased gradually because the polymer chain mobility is restricted by the presence of ImGO and a rigidified interface generates between polymer and filler. The mechanical properties have been significantly enhanced by the ImGO sheet as expected because of the presence of H-bonding. Having distinct improvement of CO 2 separation performance, the ImGO/PEBAX MMMs indicates promising applications in CO 2 capture processes." @default.
- W2344618650 created "2016-06-24" @default.
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- W2344618650 date "2016-06-01" @default.
- W2344618650 modified "2023-10-09" @default.
- W2344618650 title "Imidazole functionalized graphene oxide/PEBAX mixed matrix membranes for efficient CO2 capture" @default.
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- W2344618650 doi "https://doi.org/10.1016/j.seppur.2016.04.038" @default.
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