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- W2344670770 abstract "Understanding the mechanism of the strain-dependent conductivity change in polymers in stretched conditions is important. We observed a strain-induced growth of the conductive regions ofPSS films, induced by a coalescence of conductive PEDOT-rich cores. This growth due to coalescence leads to a gradual decrease in the electrical resistivity up to 95%, independent of the thickness of thePSS films. The primary mechanism for the evolution of the PEDOT-rich cores proceeds by the cores growing larger as they consuming relatively smaller cores. This process is caused by a strain-induced local rearrangement of PEDOT segments in the vicinity of PSS shells around the cores and also changes the chemical environment in PEDOT, induced by the electron-withdrawing effects around the PEDOT chains. The strain-induced growth mechanism is beneficial to understanding the phenomenon of polymeric chain rearrangement in mechanical deformation and to modulating the electrical conductivity for practical applications." @default.
- W2344670770 created "2016-06-24" @default.
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- W2344670770 date "2016-04-29" @default.
- W2344670770 modified "2023-10-11" @default.
- W2344670770 title "Growth Mechanism of Strain-Dependent Morphological Change in PEDOT:PSS Films" @default.
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- W2344670770 doi "https://doi.org/10.1038/srep25332" @default.
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