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- W2345528437 abstract "Functionalization of atomically thin nanomaterials enables the tailoring of their chemical, optical, and electronic properties. Exfoliated black phosphorus, a layered two-dimensional semiconductor exhibiting favorable charge carrier mobility, tunable bandgap, and highly anisotropic properties, is chemically reactive and degrades rapidly in ambient conditions. In contrast, here we show that covalent aryl diazonium functionalization suppresses the chemical degradation of exfoliated black phosphorus even following weeks of ambient exposure. This chemical modification scheme spontaneously forms phosphorus-carbon bonds, has a reaction rate sensitive to the aryl diazonium substituent, and alters the electronic properties of exfoliated black phosphorus, ultimately yielding a strong, tunable p-type doping that simultaneously improves field-effect transistor mobility and on/off current ratio. This chemical functionalization pathway controllably modifies the properties of exfoliated black phosphorus, thus improving its prospects for nanoelectronic applications." @default.
- W2345528437 created "2016-06-24" @default.
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- W2345528437 date "2016-05-02" @default.
- W2345528437 modified "2023-10-09" @default.
- W2345528437 title "Covalent functionalization and passivation of exfoliated black phosphorus via aryl diazonium chemistry" @default.
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- W2345528437 doi "https://doi.org/10.1038/nchem.2505" @default.
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