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• W2345706092 abstract "Abstract Alkali-doped fullerides show a wide range of electronic phases in function of alkali atoms and the degree of doping. Although the presence of strong electron correlations is well established, recent investigations also give evidence for dynamical Jahn–Teller instability in the insulating and the metallic trivalent fullerides. In this work, to reveal the interplay of these interactions in fullerides with even electrons, we address the electronic phase of tetravalent fulleride with accurate many-body calculations within a realistic electronic model including all basic interactions extracted from first principles. We find that the Jahn–Teller instability is always realized in these materials too. In sharp contrast to the correlated metals, tetravalent system displays uncorrelated band-insulating state despite similar interactions present in both fullerides. Our results show that the Jahn–Teller instability and the accompanying orbital disproportionation of electronic density in the degenerate lowest unoccupied molecular orbital band is a universal feature of fullerides." @default.
• W2345706092 created "2016-06-24" @default.
• W2345706092 creator A5031947762 @default.
• W2345706092 creator A5067607322 @default.
• W2345706092 date "2016-10-07" @default.
• W2345706092 modified "2023-10-16" @default.
• W2345706092 title "Orbital disproportionation of electronic density is a universal feature of alkali-doped fullerides" @default.
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• W2345706092 doi "https://doi.org/10.1038/ncomms13093" @default.
• W2345706092 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5059769" @default.
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• W2345706092 hasPublicationYear "2016" @default.
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