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• W2347052182 abstract "A cooperative photoredox and asymmetric catalysis for the enantioselective aerobic oxidative C(sp3)–H olefination of tetrahydro-β-carbolines (THCs) is reported. This method, which is also effective for tetrahydroisoquinolines (THIQs), features a triple-catalyst strategy, involving a dicyanopyrazine-derived chromophore (DPZ) as the metal-free photoredox catalyst, a chiral Lewis base catalyst, and an inorganic salt cocatalyst. The current protocol provides straightforward access to a series of valuable α-substituted THCs and THIQs in high yields with excellent regio- and enantioselectivities (up to 95% ee)." @default.
• W2347052182 created "2016-06-24" @default.
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• W2347052182 date "2016-05-10" @default.
• W2347052182 modified "2023-09-29" @default.
• W2347052182 title "Enantioselective Aerobic Oxidative C(sp³)–H Olefination of Amines via Cooperative Photoredox and Asymmetric Catalysis" @default.
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• W2347052182 doi "https://doi.org/10.1021/acscatal.6b00846" @default.
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