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- W2347492425 abstract "Ti-MCM-41 with long-ranged ordered structure was synthesized through the electrostatic interaction between positively charged surfactant micelles S~(+) and anionic silicate species I~(-)(namely electrostatic S~(+)I~(-) assembly pathway)by using the mixture of cationic surfactant C_(16)TMABr and neutral template C_nNH_(2n+3) as template. Introduction of C_nNH_(2n+3) into template influenced the structures of positively charged surfactant micelles S~(+) or liquid-crystal phases, furtherly optimized the ordered structure of Ti-MCM-41. The v_(Ti)/v_(Si) in gel, the number of carbon atoms(n) in the chain of C_nNH_(2n+3) remarkably influenced the formation of long-ranged ordered structure of Ti-MCM-41. Only when v_(Ti)/v_(Si)0.03,n18, the long-range ordered Ti-MCM-41 could be obtained. Such long-range ordered Ti-MCM-41 synthesized by mixed templating method showed the higher catalytic activity to the oxidation reactions of styrene and cyclododecene than Ti-MCM-41 synthesized by single templating route under the condition of the similiar Ti contents in Ti-MCM-41 framework." @default.
- W2347492425 created "2016-06-24" @default.
- W2347492425 creator A5035993278 @default.
- W2347492425 date "2005-01-01" @default.
- W2347492425 modified "2023-09-27" @default.
- W2347492425 title "SYNTHESIS, CHARACTERIZATION AND CATALYTIC OXIDATION PERFORMANCE OF LONG-RANGE ORDERED Ti-MCM-41" @default.
- W2347492425 hasPublicationYear "2005" @default.
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