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- W2350611801 abstract "The catalytic reduction of SO 2 with CO to elemental sulfur was considered to be the best way to get rid of SO 2 from flue gas. However, the catalyst can be poisoned by oxygen in the flue gas. In this study, with pre poisoned by SO 2, activated by O 2 CO and then sulfurized by SO 2 O 2 CO, the perovskite LaCoO 3 had excellent performance in the catalytic reduction of SO 2 with CO to elemental sulfur in the presence of 2%O 2( X (SO 2) =97%, Y (S) =95% at 500 ℃). The XRD result revealed that the perovskite structure of LaCoO 3 was unchanged after activation sulfurization, but new phases La 2O 2S and Co 3O 4 appeared. For the perovskite LaCoO 3 samples before and after activation sulfurization, the experiments of SO 2 TPD, O 2 TPD, and CO combustion in the presence of SO 2 showed that the activation sulfurization of LaCoO 3 can inhibit the formation of sulfate. At certain temperature, CO on the perovskite phase can combust with O 2 quickly, at the same time SO 2 on La 2O 2S phase can be reduced by CO, and the two reactions can be stimulated each other." @default.
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- W2350611801 date "2003-01-01" @default.
- W2350611801 modified "2023-09-25" @default.
- W2350611801 title "Reduction of sulfur dioxide with carbon monoxide over sulfurized LaCoO3 in the presence of oxygen" @default.
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