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- W2355103421 abstract "A transition metal-free catalyst composed of n-hydroxyphthalimide (nhpi), 2,3-dichloro-5,6-dicyano-benzoquinone (ddq), and nano2 was studied for the selective oxidation of alcohols using o-2 as oxidant. the reaction results showed that this catalyst system can effectively catalyze the oxidation of alcohols to the corresponding aldehydes or ketones. 99% selectivity for benzaldehyde at 65% conversion of benzyl alcohol was obtained at 80 degrees c for 6 h. in the process of reaction, ddq abstracted a hydrogen atom from nhpi to generate a highly reactive pino free radical and hydroquinone. then, pino abstracted a hydrogen atom from alcohols to generate aldehydes or ketones. finally, no from nano2 decomposition in the reaction media catalyzed the oxidation of hydroquinone to quinone by o-2." @default.
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- W2355103421 date "2011-01-01" @default.
- W2355103421 modified "2023-09-26" @default.
- W2355103421 title "Selective Oxidation of Alcohols Catalyzed by a Transition Metal-Free System of NHPI/DDQ/NaNO2" @default.
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