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- W2360223170 abstract "Global kinetics of isoprene selective hydrogenation over the commercial Ni-Mo/Al2O3 catalyst was investigated by using an integral fixed bed reactor.The influences of reaction temperature,reaction pressure,hydrogen/oil volume ratio and liquid hourly space velocity on the selective hydrogenation reaction were studied by using the isoprene + n-octane solution as model feed and under following conditions: reaction temperature 70~120℃,reaction pressure 0.5~2.0 MPa,liquid hourly space velocity 2~36 h·1 and hydrogen/ oil volume ratio 20~40.A power-law kinetic model was used to describe the global kinetics of the series reaction of isoprene selective hydrogenation.The results show that the reaction activation energy of isoprene hydrogenation to isopentene is 44.3 kJ·mol-1,and the reaction orders with respect to isoprene and hydrogen are 0.98 and 0.27,respectively;the reaction activation energy of isopentene hydrogenation to isopentane is 101.1 kJ·mol-1,the reaction orders with respect to isopentene and hydrogen are 1.57 and 1.09,respectively.The statistical test and the comparison of the isoprene conversion ratio and isopentene selectivity obtained by experiments to those obtained by the calculation results of the model indicate that the model used is reliable." @default.
- W2360223170 created "2016-06-24" @default.
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- W2360223170 date "2011-01-01" @default.
- W2360223170 modified "2023-09-27" @default.
- W2360223170 title "Global Kinetics of Isoprene Selective Hydrogenation over the Commercial Ni-Mo/Al_2O_3 Catalyst" @default.
- W2360223170 hasPublicationYear "2011" @default.
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