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- W2361704299 abstract "The standard heat of formation ΔfHm0,entropy Sm0 and heat capacity Cp,m of the possible compounds involved in the re-action system of cyclohexene,ethylene,carbon dioxide and hydrogen were calculated by Benson group contribution method.The Gibbs free energy and equilibrium constants of the possible reactions of above system were calculated and used to forecast the feasi-bility and the extent of reactions.The effects of temperature and pressure on the reactions were discussed.The results revealed that lower temperature and higher pressure are favorable to all reactions.The hydrogenation of carbon dioxide to carbon monoxide or formic acid,and hydrogenation of carboxylic acids to aldehydes were thermodynamically unfavorable.While hydrogenation of alkenes to alkanes,hydrogenation of aldehydes to alcohols,and formation of carboxylic acids or aldehydes from the reactions of alkenes with carbon dioxide or carbon monoxide were thermodynamically favorable within certain range of temperature.From the thermodynamic view,the structure of alkene had great effects on the above reactions and ethylene was more easily hydrofomylated than cyclohexene." @default.
- W2361704299 created "2016-06-24" @default.
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- W2361704299 date "2010-01-01" @default.
- W2361704299 modified "2023-09-23" @default.
- W2361704299 title "Thermodynamic analysis of reaction system of olefins,carbon dioxide and hydrogen" @default.
- W2361704299 hasPublicationYear "2010" @default.
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