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- W2365892307 abstract "On the basis of experiments, thermodynamic analysis for vapor phase carbonylation of methanol to acetic acid over Ni/AC catalyst at atmospheric pressure, with referring to the liquid phase and pressurized vapor phase carbonylation path and mechanism, was carried out, and the path and mechanism of the system were discussed. It is shown that the possible intermediate CH 3CO-Ni 2+ -I species can not be reduced directly to zero valent nickel to release acetyl iodide, and all carbonylation steps may be implemented through CH 3CO-Ni 2+ -I species. Besides methyl acetate hydrolysis,the direct reaction between methanol and CH 3CO-Ni 2+ -I species may also play a role in the formation of acetic. Dimethyl ether is mainly produced over the activated carbon carrier through the dehydation of methanol which is catalyzed by both activated carbon and methyl iodide with catalytic step of nickel, but not through the direct reaction between methanol and methyl iodide. The thermodynamic analysis of the system suggests that the productivity of acetic acid would be improved when water steam is added into the feed flow of the system." @default.
- W2365892307 created "2016-06-24" @default.
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- W2365892307 date "2002-01-01" @default.
- W2365892307 modified "2023-09-25" @default.
- W2365892307 title "Thermodynamic analysis on vapor-phase carbonylation of methanol to acetic acid over Ni/AC catalyst" @default.
- W2365892307 hasPublicationYear "2002" @default.
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