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- W2368851580 abstract "The decomposition reaction kinetics of gun propellant TG0604 was investigated by non-isothermal method with TG-DTG under atmospheric pressure and ambulatory atmosphere conditions.The results show that there are two reaction stages in the decomposition process of gun propellant TG0604.The decomposition reaction mechanism of stage I obeys Mample single-file law with n=1,the kinetic parameters are obtained as: Ea=79.09kJ·mol-1,A=107.40s-1,and the kinetic equations can be expressed as:dα/dt=107.40(1-α)e-0.95×104/T;The decomposition reaction mechanism of stage II obeys three-step chemical reaction rule,the kinetic parameters are obtained as: Ea=214.79kJ·mol-1,A=1021.49s-1 and the kinetic equations can be expressed as:dα/dt=1021.19(1-α)3e-2.58×104/T.The critical temperatures of thermal explosion of gun propellant TG0604 obtained from the onset temperature(Te) and the peak temperature(Tp) are: Tbe=461.51K,Tbp=478.17K.ΔS≠,ΔH≠ and ΔG≠ of the two stages are calculated as: for stage I,-86.70J·mol-1·K-1,80.54kJ·mol-1 and 417.98kJ·mol-1;for stage II,214.78J·mol-1·K-1,236.95kJ·mol-1 and 136.07kJ·mol-1." @default.
- W2368851580 created "2016-06-24" @default.
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- W2368851580 date "2007-01-01" @default.
- W2368851580 modified "2023-09-24" @default.
- W2368851580 title "Non-isothermal Thermal Decomposition Reaction Kinetics of TEGDN Gun Propellant" @default.
- W2368851580 hasPublicationYear "2007" @default.
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