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- W2372743164 abstract "Abstract Interactions between a poly(vinyl)silazane and Al 2 O 3 or Y 2 O 3 -stabilised ZrO 2 fillers were studied during the fabrication of polysilazane-derived bulk ceramics in order to investigate the influence of oxide fillers on resulting properties. Specimens were produced by coating of the filler powders with the polysilazane, warm-pressing of the resulting composite powders, and pyrolytic conversion in flowing N 2 at various temperatures between 1000 °C and 1400 °C. Significant differences in densification were observed, depending on the filler used. Reactions between the polysilazane-derived matrix and Al 2 O 3 or ZrO 2 at temperatures ≥1300 °C resulted in the formation of Si 5 AlON 7 or ZrSiO 4 , respectively. Reactivity in the polysilazane-derived component was a result of SiO 2 contamination caused primarily by adsorbed species on the filler particle surface. Knowledge of polysilazane/filler interface processes is found to be decisive for the prediction of properties such as shrinkage and porosity, which heavily influence performance of a material." @default.
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- W2372743164 date "2011-12-01" @default.
- W2372743164 modified "2023-09-27" @default.
- W2372743164 title "Matrix–filler interactions in polysilazane-derived ceramics with Al2O3 and ZrO2 fillers" @default.
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- W2372743164 doi "https://doi.org/10.1016/j.jeurceramsoc.2011.07.015" @default.
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