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- W2373508743 abstract "In order to study the catalysis of tetra(4-carboxylphenyl) porphyrin supported on ZnO for aerobic oxidation of toluene under mild conditions and in the absence of any solvent and reductant,ZnO supported tetra(4-carboxylpheny1) porphyrin(Co TCPP/ZnO) was prepared by the method of precipitation and calcinations,and characterized by UV-Vis,FT-IR and XRD spectroscopic techniques.The results show that a quantity of catalyst containing only 1.89×10-6 mol of Co TCPP could be efficiently reused 11 times for the oxidation of toluene,with 6.84% toluene conversion rate,50.47% selectivity for aldehyde and alcohol,and a catalyst turnover number of 6.52×104,on average,under the optimal reaction conditions of 180 ℃ and 0.6 MPa.It was found that ZnO supported catalyst was more effective and reusable for the oxidation of toluene than the unsupported catalyst.The research results confirm that ZnO has a good promotion for the catalysis of Co TCPP for the oxidation of toluene and protect Co TCPP from oxidation destruction by O2." @default.
- W2373508743 created "2016-06-24" @default.
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- W2373508743 date "2012-01-01" @default.
- W2373508743 modified "2023-10-16" @default.
- W2373508743 title "Catalytic performance of ZnO supported cobalt tetra(4-carboxylphenyl)porphyrin" @default.
- W2373508743 hasPublicationYear "2012" @default.
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