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- W237453114 abstract "The third-order optical susceptibility ${ensuremath{chi}}^{(3)}$ of polyacetylene is calculated by the Lanczos-based density-matrix renormalization group. The theoretical results now remarkably agree with two different sets of experimental data: both the positions of two major peaks and their relative intensities. The 0.89 eV peak, originally assigned to a two-photon resonance, is actually a three-photon resonance due to the ${mathrm{nB}}_{u}$ state. This state lies above the band-edge state ${mathrm{jB}}_{u}$ which itself accounts for a hidden hump on the right shoulder of the 0.6 eV peak. The electron correlation effect is the main origin of these rich features." @default.
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- W237453114 title "Origin of the 0.89 eV peak in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mi>χ</mml:mi></mml:mrow><mml:mrow><mml:mn /><mml:mo>(</mml:mo><mml:mn>3</mml:mn><mml:mo>)</mml:mo><mml:mn /></mml:mrow></mml:msup></mml:mrow><mml:mo>(</mml:mo><mml:mi>−</mml:mi><mml:mn>3</mml:mn><mml:mi>ω</mml:mi><mml:mo>;</mml:mo><mml:mi>ω</mml:mi><mml:mo>,</mml:mo><mml:mi>ω</mml:mi><mml:mo>,</mml:mo><mml:mi>ω</mml:mi><mml:mo>)</mml:mo></mml:math>of …" @default.
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- W237453114 doi "https://doi.org/10.1103/physrevb.61.4377" @default.
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