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- W2377713053 abstract "MoOx-LaHY catalysts were prepared with the mixture of(NH4)6Mo7O24·4H2O and LaHY through solid-state reaction under air atmosphere and characterized by XRD and NH3-TPD techniques;their hydrodesulfurization(HDS) performance was evaluated by using the solution of dibenzothiophene(DBT,0.6% by mass) in decane as a model reactant.The results indicated that by using solid-state reaction at 520℃,4.36% of Mo species is incorporated into the molecular sieve LaHY,which forms the single-phase complex nMoOx·LaHY,while the rest Mo species is dispersed on the outer surface of LaHY.As a result of forming the single-phase complex,the lattice parameters of MoOx-LaHY catalysts are enlarged and their acidity is reduced.Over the sulfided MoOx-LaHY catalysts,the conversion of DBT reaches 86.74% for the HDS under the conditions of 310℃,4.0MPa and a space velocity 20h-1.Raising the solid-state reaction temperature may increase the content of the single-phase complex incorporated in the resultant MoOx-LaHY catalysts,but it cannot significantly enhance their HDS activity." @default.
- W2377713053 created "2016-06-24" @default.
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- W2377713053 date "2011-01-01" @default.
- W2377713053 modified "2023-09-23" @default.
- W2377713053 title "Hydrodesulfurization performance of MoO_3-LaHY catalyst prepared by solid-state reaction" @default.
- W2377713053 hasPublicationYear "2011" @default.
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