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- W2380901863 abstract "The complete high-order perturbation formula of g factor for 3d(3) ions in cubic octahedral site was derived. In the formula, both the contribution delta g(CF) to g-shift delta g (= g-g(s), where g(s) = 2.0023) due to crystal-field (CF) mechanism (related to the interactions of CF excited states with the ground state) and that (delta g(CT)) due to charge-transfer (CT) mechanism (related to the interactions of CT excited states with the ground state, which is omitted in crystal-field theory) are included. By using the formula and the parameters obtained from the optical spectra of CaZrO3:Mn4+ crystal, the g factor of CaZrO3:Mn4+ was calculated. The result is consistent with the experimental value. The calculations show that the contribution is opposite in sign and about 62% in magnitude compared with the contribution delta g(CF). It appears that both CF and CT mechanisms should be considered in the calculation of g factor for the high valence 3d(3) (e. g. , Mn4+ and Fe3+) ions in crystals." @default.
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- W2380901863 date "2008-08-01" @default.
- W2380901863 modified "2023-09-27" @default.
- W2380901863 title "[Studies of the g factor and optical spectra for CaZrO3:Mn4+ crystal]." @default.
- W2380901863 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18975784" @default.
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