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- W2384123090 abstract "Gas chromatography has been used to determine the concentration of dibutyl phosphate(DBP)and monobutyl phosphate(MBP)produced fromα-radiolysis due to 238Pu in the 30%TBP-kerosene-HNO3extraction system.The effects of back-extractant,stripping conditions and concentration of plutonium were studied on the concentration of DBP and MBP.Moreover,the effects of total dose,nitric acid concentration,dose rate and dilutes on the concentration of DBP and MBP were investigated.The results show that the concentration of DBP and MBP increases with absorbed dose and dose rate.When the absorbed dose is 5×104 Gy and the absorbed dose rate is 73.7Gy/min,among n-dodecane,hydrogenation kerosene and special kerosene,the yields of DBP are 4.45×10-2 mol/L,4.44× 10-2 mol/L,4.35×10-2 mol/L,respectively,and the yields of MBP are 3.52×10-3 mol/L,3.52×10-3 mol/L,3.50×10-3 mol/L,respectively.When the absorbed dose increases to 5×105 Gy,the concentration of DBP and MBP in three dilutes are approximately equal.When the absorbed dose is 5×104 Gy,the concentrations of DBP and MBP in system of α-radiolysis are 5.57×10-2 mol/L and 5.10×10-3 mol/L respectively,the corresponding concentration of DBP and MBP in system ofγ-radiolysis are 2.50×10-3 mol/L and 3.14× 10-4 mol/L respectively,the concentrations of DBP and MBP produced fromα-radiolysis of extraction system are obviously greater than those fromγ-radiolysis of system at same dose." @default.
- W2384123090 created "2016-06-24" @default.
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- W2384123090 date "2013-01-01" @default.
- W2384123090 modified "2023-09-26" @default.
- W2384123090 title "α-Radiolysis Behaviour of 30%TBP-Kerosene-HNO_3 Extraction System I.Analysis of DBP and MBP in Radiolytic Products" @default.
- W2384123090 hasPublicationYear "2013" @default.
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