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- W2386396345 abstract "Pd catalysts supported on mesoporous alumina (M-Al2O3) were prepared by an impregnation method and tested for CH4 catalytic combustion. PdO/M-Al2O3 was more active than the PdO catalyst supported on conventional Al2O3 because of a higher dispersion of PdO species induced by the mesoporous structure of M-Al2O3. Moreover, with increasing calcination temperature, the conversion of CH4 over PdO/M-Al2O3 catalysts first increased and then decreased. The best catalytic performance was obtained on the PdO/M-Al2O3 catalyst calcined at 700 oC, with a CH4 conversion of 91% at 400 oC. Pd species were mainly in mesoporous channels of the support in the form of highly dispersed PdO particles. When calcined at higher temperature, Pd species were in forms of crystalline Pd and PdO. A decline of reactivity and a higher turnover frequency were obtained on the PdO/M-Al2O3 catalyst calcined at 900 oC, which might be due to the co-existence of metallic Pd and PdO in the catalyst." @default.
- W2386396345 created "2016-06-24" @default.
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- W2386396345 date "2011-01-01" @default.
- W2386396345 modified "2023-09-27" @default.
- W2386396345 title "Mesoporous Alumina Supported PdO Catalysts for Catalytic Combustion of Methane" @default.
- W2386396345 hasPublicationYear "2011" @default.
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