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- W2389746871 abstract "In order to investigate the relationship between the composition and the activity of Mn-Ce-O composites, 7 samples with Mn/Ce molar ratios of 10/0, 8/2, 6/4, 5/5, 4/6, 2/8, 0/10 were prepared by co-precipitation. NH3 was selected as a model pollutant and H2O2 was used as oxidant. The oxidation reaction in supercritical water was carried out in a continuous flow packed-bed reactor at th temperature of 450 ℃, the pressure of 25 MPa, and the residence time of 1 s with the oxidant addition of 2.94 times the stoichiometric amount. The catalytic activity is greatly influenced by the catalyst composition and the catalyst with Mn/Ce mol ratio of 5/5 is found to be the best one, on which the conversion of NH3 can reach to 99.7%. The catalysts were characterized by N2 adsorption, XRD and TPR. The results indicate that there exists an interaction between Mn and Ce oxides." @default.
- W2389746871 created "2016-06-24" @default.
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- W2389746871 date "2007-01-01" @default.
- W2389746871 modified "2023-09-25" @default.
- W2389746871 title "Composition-activity effect of Mn-Ce-O composites on NH_3 catalytic supercritical water oxidation" @default.
- W2389746871 hasPublicationYear "2007" @default.
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