Matches in SemOpenAlex for { <https://semopenalex.org/work/W2393949105> ?p ?o ?g. }
- W2393949105 endingPage "4063" @default.
- W2393949105 startingPage "4047" @default.
- W2393949105 abstract "Sn-β zeolites prepared using different recipes feature very different catalytic activities for aqueous phase glucose isomerization, suggesting the presence of different active sites. A systematic study of the morphology and atomic-level structure of the materials using DNP NMR spectroscopy in combination with first-principles calculations allows for the discrimination between potential sites and leads to a proposal of specific structural features that are important for high activity. The results indicate that the materials showing the highest activity possess a highly hydrophobic, defect-free zeolite framework. Those materials show so-called closed and associated partially hydrolyzed Sn(IV) sites in the T6 and T5/T7 lattice positions. On the other hand, postsynthetically synthesized Sn-β samples prepared in two steps via dealumination and subsequent solid-state ion exchange from Al-β show significantly lower activity, which is associated with a hydrophilic framework and/or a lower accessibility and differ..." @default.
- W2393949105 created "2016-06-24" @default.
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- W2393949105 date "2016-05-26" @default.
- W2393949105 modified "2023-10-13" @default.
- W2393949105 title "Correlating Synthetic Methods, Morphology, Atomic-Level Structure, and Catalytic Activity of Sn-β Catalysts" @default.
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