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• W2396676410 abstract "Relativistic four-component random phase approximation (RPA) calculations of indirect nuclear spin–spin coupling constants in MH4 (M=C, Si, Ge, Sn, Pb) and Pb(CH3)3H are presented. The need for tight s-functions also in relativistic four-component calculations is verified and explained, and the effect of omission of (SS–LL) and (SS–SS) two-electron integrals is investigated. Already in GeH4 we see a relativistic increase in the coupling constant by 12%, and for PbH4 the effect is a 156% increase for the one-bond coupling. Large relativistic effects are also computed for the two-bonds couplings. We find that the relativistic effects on the one-bond couplings are mainly due to scalar relativistic factors rather than spin–orbit corrections." @default.
• W2396676410 created "2016-06-24" @default.
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• W2396676410 date "2000-02-22" @default.
• W2396676410 modified "2023-09-23" @default.
• W2396676410 title "Relativistic four-component calculations of indirect nuclear spin–spin couplings in MH4 (M=C, Si, Ge, Sn, Pb) and Pb(CH3)3H" @default.
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• W2396676410 doi "https://doi.org/10.1063/1.480504" @default.
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