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- W2396885685 abstract "The influence of SO2 on Hg0 removal behavior over CeO2–TiO2 (CeTi) adsorbent prepared by a sol–gel method was investigated at low temperature. The fresh, sulfated, and used materials were well characterized by means of N2 physisorption, X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), Raman, hydrogen gas temperature–programmed reduction (H2–TPR), thermal gravimetric and differential scanning calorimetry (TG–DSC), and X-ray photoelectron spectroscopy (XPS) techniques to illustrate the promotional mechanism of SO2 on Hg0 removal. The results indicated that in the initial reaction period, the Hg0 removal efficiency significantly increased with the presence of SO2 because of the reaction between CeTi and SO2. With the sulfation time increasing, the promotional effect of SO2 on Hg0 removal over CeTi adsorbent gradually decreased due to the presence of large amount of cerium sulfate species. The Hg0 removal efficiency over CeTi first increased with the reaction temperature increasing, and then decreased with further temperature rising above 150 °C. The reducibility of CeTi significantly decreased after sulfation, while the sulfation led to an enhancement of the Ce3+ content formed on the adsorbent surface. In the process of Hg0 removal with SO2 presence, the redox couple of [CeO2 (Ce4+) ↔ Ce2O3 (Ce3+)] played a significant role in Hg0 removal to proceed, and SO2 made an important contribution to this redox process." @default.
- W2396885685 created "2016-06-24" @default.
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- W2396885685 date "2016-09-01" @default.
- W2396885685 modified "2023-10-16" @default.
- W2396885685 title "Promotional effect of SO 2 on CeO 2 –TiO 2 material for elemental mercury removal at low temperature" @default.
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- W2396885685 doi "https://doi.org/10.1016/j.apr.2016.05.003" @default.
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