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- W2401303709 abstract "Multi-hierarchy self-assembly (MHSA) is one of the key processes responsible for the spontaneous formation of a broad variety of complex structures. However, because of its complexity, the mechanism of this process remains unknown in most cases. Thus, a deeper understanding of MHSA is needed, especially for the preparation of MHSA systems via bottomup methodologies. We show here, experimentally and theoretically, that the complex-formation MHSA of peptide nanotube films can be controlled by a single experimental parameter the humidity. Furthermore, we identify growth-front nucleation (GFN: formation of new grains at the perimeter) as the physical background for the observed morphological transitions by correlating the experimental observations with phase-field modelling of morphological evolution. Our findings indicate that there is a simple way to control multi-hierarchy morphologies, a finding crucial for employing bottom-up techniques in constructing complex structures for practical applications." @default.
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- W2401303709 date "2015-01-01" @default.
- W2401303709 modified "2023-09-27" @default.
- W2401303709 title "Controlling the growth forms of peptide-nanotube spherulitic films: experiments and simulations" @default.
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