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• W2410130782 endingPage "3968" @default.
• W2410130782 startingPage "3961" @default.
• W2410130782 abstract "On the basis of a temperature-induced effect, the solvothermal reaction of Co(Ac)2·4H2O, 5-amino-2,4,6-triiodoisophthalic acid (H2atibdc), and 1,4-bis(2-methyl-imidazol-1-yl)butane (bib) at 80 °C gave a new coordination polymer [Co(bib)(atibdc)] (1), which shows a two-dimensional (2D) network with left- and right-handed helical chains. By raising the reaction temperature to 130 °C, a pair of homochiral enantiomers [Co(bib)(atibdc)]·2H2O (2, 2M, and 2P) were successfully obtained, displaying a three-dimensional (3D) framework with three kinds of unique helical chains. Keeping the temperature of the reaction system to 150 °C, excited, an in situ iodine elimination reaction occurred, and a new linker 5-aminoisophthalic acid (H2aipa) was generated, which then cooperated with the bib ligand to construct a coordination polymer [Co(bib)(aipa)] (3), showing a 3D 3-fold interpenetrating architecture. The comparison of final solid structures exhibits an exclusive temperature-induced effect on the construction of the coordination polymer. Furthermore, via a single-crystal-to-single-crystal (SCSC) transformation, the 2D network of 1 can be derived from the 3D framework of 2, which presents a rare type of temperature-solvent induced SCSC transformation. In addition, the magnetic properties of 1–3 have been investigated as well." @default.
• W2410130782 created "2016-06-24" @default.
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• W2410130782 creator A5051153382 @default.
• W2410130782 date "2016-06-09" @default.
• W2410130782 modified "2023-10-15" @default.
• W2410130782 title "Temperature-Induced Syntheses, Iodine Elimination, Enantiomers Resolution, and Single-Crystal-to-Single-Crystal Transformation of Imidazole-Co(II) Coordination Polymers with Amino-isophthalic Acid as Co-Ligand" @default.
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• W2410130782 doi "https://doi.org/10.1021/acs.cgd.6b00527" @default.
• W2410130782 hasPublicationYear "2016" @default.
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