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- W2410369990 abstract "Time-resolved electron diffraction with atomic-scale spatial and temporal resolution was used to unravel the transformation pathway in the photoinduced structural phase transition of vanadium dioxide. Results from bulk crystals and single-crystalline thin-films reveal a common, stepwise mechanism: First, there is a femtosecond V-V bond dilation within 300 fs, second, an intracell adjustment in picoseconds and, third, a nanoscale shear motion within tens of picoseconds. Experiments at different ambient temperatures and pump laser fluences reveal a temperature-dependent excitation threshold required to trigger the transitional reaction path of the atomic motions." @default.
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- W2410369990 date "2016-05-01" @default.
- W2410369990 modified "2023-10-16" @default.
- W2410369990 title "Ultrafast electron crystallography of the cooperative reaction path in vanadium dioxide" @default.
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- W2410369990 doi "https://doi.org/10.1063/1.4953370" @default.
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