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• W2414086594 abstract "The entropic effects in the comicellization behavior of amphiphilic $AB$ copolymers differing in the chain size of solvophilic $A$ parts were studied by means of molecular dynamics simulations. In particular, mixtures of miktoarm star copolymers differing in the molecular weight of solvophilic arms were investigated. We found that the critical micelle concentration values show a positive deviation from the analytical predictions of the molecular theory of comicellization for chemically identical copolymers. This can be attributed to the effective interactions between copolymers originated from the arm size asymmetry. The effective interactions induce a very small decrease in the aggregation number of preferential micelles triggering the nonrandom mixing between the solvophilic moieties in the corona. Additionally, in order to specify how the chain architecture affects the size distribution and the shape of mixed micelles we studied star-shaped, H-shaped, and homo-linked-rings--linear mixtures. In the first case the individual constituents form micelles with preferential and wide aggregation numbers and in the latter case the individual constituents form wormlike and spherical micelles." @default.
• W2414086594 created "2016-06-24" @default.
• W2414086594 creator A5004821943 @default.
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• W2414086594 date "2015-11-20" @default.
• W2414086594 modified "2023-09-25" @default.
• W2414086594 title "Entropic effects, shape, and size of mixed micelles formed by copolymers with complex architectures" @default.
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• W2414086594 doi "https://doi.org/10.1103/physreve.92.052601" @default.
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• W2414086594 hasPublicationYear "2015" @default.
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