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• W2414347796 endingPage "9926" @default.
• W2414347796 startingPage "9922" @default.
• W2414347796 abstract "By judiciously modulating the ring strain and sterics, we developed a class of disubstituted cyclopropenes that selectively underwent single monomer addition in ring-opening metathesis but readily underwent alternating ring-opening metathesis polymerization with low-strain cyclic olefins in a living fashion. The substituents on cyclopropenes effectively inhibited homoaddition and prevented secondary metathesis on the polymer backbone. The resulting polymers had controllable molecular weights and end groups, very low dispersities, and high regularity in microstructure under optimized conditions. 1H and 13C NMR spectroscopy and MALDI-TOF MS showed a rigorously alternating sequence. Interestingly, disubstituted cyclopropenes were found to present zero-order kinetics, indicating their rapid single addition and the rate-determining ring opening of the low-strain olefin." @default.
• W2414347796 created "2016-06-24" @default.
• W2414347796 creator A5046992236 @default.
• W2414347796 creator A5075565259 @default.
• W2414347796 date "2015-07-30" @default.
• W2414347796 modified "2023-10-01" @default.
• W2414347796 title "Living Alternating Ring-Opening Metathesis Polymerization Based on Single Monomer Additions" @default.
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• W2414347796 doi "https://doi.org/10.1021/jacs.5b05497" @default.
• W2414347796 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26182144" @default.
• W2414347796 hasPublicationYear "2015" @default.
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