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• W2416221270 endingPage "65" @default.
• W2416221270 startingPage "59" @default.
• W2416221270 abstract "In this work, we synthesized tantalum (Ta) nanoclusters on carbon black (Ta/CB) via simple electrodeposition in non-aqueous solvent, acetonitrile (ACN) at ambient temperature. Transmission electron microscopy (TEM) images showed that the electrodeposited Ta nanoclusters consisted of tiny Ta nanoparticles. X-ray photoelectron spectroscopy (XPS) result represented that the outermost Ta formed the native oxide on Ta/CB due to its ambient exposure to air. Electrochemical catalytic properties of prepared Ta/CB on glassy carbon electrode (Ta/CB/GC) were investigated toward reductions of oxygen and hydrogen peroxide, and oxidations of ascorbic acid and dopamine. For oxygen reduction reaction (ORR) in acid, Ta/CB/GC represented a decent electrocatalytic performance which was better or comparable to bare Pt. The operational stability in acidic condition was maintained up to 500 repetitive potential cycles presumably due to the protective native Ta oxide layer. Ta/CB/GC also showed high amperometric sensitivity (4.5 (±0.16) mA mM(-1) cm(-2), n = 5) for reduction of hydrogen peroxide in 0.1 M phosphate buffer solution (PBS, pH 7.4). In addition, Ta/CB/GC was demonstrated for the possibility of simultaneous detection of ascorbic acid and dopamine using differential pulse voltammetry (DPV)." @default.
• W2416221270 created "2016-06-24" @default.
• W2416221270 creator A5000806138 @default.
• W2416221270 creator A5051864897 @default.
• W2416221270 creator A5058177669 @default.
• W2416221270 date "2016-08-01" @default.
• W2416221270 modified "2023-10-14" @default.
• W2416221270 title "Electrodeposition of tantalum on carbon black in non-aqueous solution and its electrocatalytic properties" @default.
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• W2416221270 doi "https://doi.org/10.1016/j.aca.2016.05.030" @default.
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