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• W2417442466 abstract "The diverse applications of acrylate metathesis range from synthesis of high-value α,β-unsaturated esters to depolymerization of unsaturated polymers. Examined here are unexpected side reactions promoted by the important Grubbs catalyst GII. Evidence is presented for attack of PCy3 on the acrylate olefin to generate a reactive carbanion, which participates in multiple pathways, including further Michael addition, proton abstraction, and catalyst deactivation. Related chemistry may be anticipated whenever labile metal–phosphine complexes are used to catalyze reactions of substrates bearing an electron-deficient olefin." @default.
• W2417442466 created "2016-06-24" @default.
• W2417442466 creator A5010060889 @default.
• W2417442466 creator A5077537923 @default.
• W2417442466 date "2015-06-05" @default.
• W2417442466 modified "2023-09-27" @default.
• W2417442466 title "Acrylate Metathesis via the Second-Generation Grubbs Catalyst: Unexpected Pathways Enabled by a PCy₃-Generated Enolate" @default.
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• W2417442466 doi "https://doi.org/10.1021/jacs.5b04524" @default.
• W2417442466 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26030596" @default.
• W2417442466 hasPublicationYear "2015" @default.
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