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• W2418771097 abstract "We introduce a general kinetic model for crystal dissolution that explicitly tracks all the various atoms in the crystal structure as part of the reaction mechanism. This model will be used in this and subsequent articles to develop a theory for the treatment of experimental and field water-rock kinetic data. The model is based on a many-body reaction mechanism. It is built from both elementary reactions, i.e., bond-breaking and bond-forming, and basic reactions, i.e., dissolution of surface units, adsorption and incorporation of solution units, and mobility of units at the crystal surface. The full crystal structure is used to calculate the interactions of neighboring atoms as well as possible defects of the crystal lattice in the model. This approach is different from models based on either molecular precursor complexes or adsorption." @default.
• W2418771097 created "2016-06-24" @default.
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• W2418771097 date "2004-04-01" @default.
• W2418771097 modified "2023-10-17" @default.
• W2418771097 title "Mineralogical approaches to fundamental crystal dissolution kinetics" @default.
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• W2418771097 doi "https://doi.org/10.2138/am-2004-0407" @default.
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