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• W2419048032 startingPage "12082" @default.
• W2419048032 abstract "The concept of hydrogen storage via liquid organic hydrides in cycles of hydrogenation and dehydrogenation with preferably low amount of reaction enthalpy is well known under the abbreviation LOHC, Liquid Organic Hydrogen Carrier. However, our study addresses the dehydrogenation of methylcyclohexane in a prototype microstructured membrane reactor, which is mainly devoted to the heat storage in a so-called LORC, a Liquid Organic Reaction Cycle. While using the same cycles of hydrogenation and dehydrogenation, heat shall be stored on the contrary by high reaction enthalpy in the LORC. A novel planar membrane module with an integrated catalytic fixed-bed has been developed. It is equipped with structured supports to reduce the mechanical stress on the Pd-membrane foil. Experiments investigating the membrane separation performance were conducted with operational parameters up to 400 °C and 13 bar. The ability of shifting equilibrium conditions to product side and pure H2 recovery was shown. Catalyst deactivation and regeneration was tested in order to analyze stability of the Pd-membrane. An experimental parameter study was performed to obtain a future optimized design of a large-scale prototype reactor." @default.
• W2419048032 created "2016-06-24" @default.
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• W2419048032 date "2016-07-01" @default.
• W2419048032 modified "2023-10-14" @default.
• W2419048032 title "Heat storage by the dehydrogenation of methylcyclohexane – Experimental studies for the design of a microstructured membrane reactor" @default.
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• W2419048032 doi "https://doi.org/10.1016/j.ijhydene.2016.05.140" @default.
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