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- W2419981046 abstract "Preparation of molybdenum dioxido complexes with novel iminophenolate ligands bearing pendant secondary amide functionalities led to unprecedented C-C and C-N coupling reactions of two α-iminoamides upon coordination. The diastereoselective cyclization to asymmetric imidazolidines occurs at the metal center in two consecutive steps via a monocoupled intermediate. A meaningful mechanism is proposed on the basis of full characterization of intermediate and final molybdenum-containing products by spectroscopic means and by single-crystal X-ray diffraction analyses. This process constitutes the first example of a diastereoselective self-cyclization of two α-iminoamides." @default.
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- W2419981046 date "2015-12-08" @default.
- W2419981046 modified "2023-09-26" @default.
- W2419981046 title "Templated C–C and C–N Bond Formation Facilitated by a Molybdenum(VI) Metal Center" @default.
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- W2419981046 doi "https://doi.org/10.1021/acs.inorgchem.5b02347" @default.
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