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• W2425485514 startingPage "3767" @default.
• W2425485514 abstract "High-resolution 1s near-edge spectra of molecular nitrogen and variable size nitrogen clusters obtained using monochromatic synchrotron radiation from the high brilliance BESSY-II storage ring facility are reported. The vibrationally resolved $1{ensuremath{sigma}}_{u}ensuremath{rightarrow}1{ensuremath{pi}}_{g}$ core-to-valence excitation band of clusters shows a distinct redshift of $6ifmmodepmelsetextpmfi{}1mathrm{meV}$ relative to the isolated molecule, but the vibrational structure and linewidths are essentially unchanged. This shift is assigned to dynamic stabilization of $1{ensuremath{sigma}}_{u}ensuremath{rightarrow}1{ensuremath{pi}}_{g}$ excited molecules in clusters, arising from the dynamic dipole moment generated by core-hole localization in the low-symmetry cluster field. This leads to changes in intermolecular interactions compared to the ground-state cluster. Such spectral shifts are expected to occur generally in molecular clusters and in the corresponding condensed phase." @default.
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• W2425485514 date "2001-04-23" @default.
• W2425485514 modified "2023-10-18" @default.
• W2425485514 title "Dynamic Stabilization in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mn>1</mml:mn><mml:mi>σ</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant=italic>u</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mo>→</mml:mo><mml:mrow><mml:msub><mml:mrow><mml:mn>1</mml:mn><mml:mi>π</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant=italic>g</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math>Excited Nitrogen Clusters" @default.
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• W2425485514 doi "https://doi.org/10.1103/physrevlett.86.3767" @default.
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