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- W243191293 abstract "Two basic ways of applying biochemical reactions in electrochemical current sources which are outlined are (1) creation of fuel cells that utilize the products of enzymatic cleavage of complex organic substances as the fuel and (2) use of enzymes as heterogeneous catalysts accelerating the transport of electrons from fuel (or an oxidizing agent) to the electrode, which should provide for an increase in the power of the cells per unit volume or weight. A system is described in which oxidation of hydrogen and generation of the electrochemical potential occur on a pyrographite electrode with the participation of an enzyme with hydrogenase action. The transfer of electrons from the active site of the enzyme to the electrode occurs with the aid of the mediator methylviologen. The kinetics and equilibrium of the reaction of methylviologen were investigated. Results of experiments at various pH values permitted an estimation of the equilibrium constant. The electrochemical reduction and oxidation of methylviologen on the pyrographite electrode was investigated. (BLM)" @default.
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- W243191293 date "1975-11-01" @default.
- W243191293 modified "2023-09-24" @default.
- W243191293 title "Biochemical fuel cells. Hydrogenase as a catalyst of the oxidation of hydrogen in the mediator: carbon electrode system. [Methylviologen mediator]" @default.
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