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- W243457578 abstract "The objective of this work is to study the chemistry and reaction mechanism of species resulting from the pyrolysis of coal particles. Emphasis is placed on clarifying and understanding coal chemistry during the early initial steps of coal gasification where highly reactive gas phase intermediate species can be observed by rapidly bringing the coal to reaction temperature. The experiments are designed such that reactive gas phase intermediates can leave the reaction zone without wall collisions and be trapped with an inert gas on a cold (12/sup 0/K) matrix surface. Identification and characterization of these gaseous species and possibly free radicals are performed in a newly designed matrix isolation system coupled to a high resolution Fourier Transform I.R. Variables such as temperature, coal particle size, heating technique, tar formation, and addition of isotopically enriched reactant species were studied. Structural data of coal from fluorocoal and polycyclic aromatic model compounds were also pursued. 23 refs., 48 figs." @default.
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- W243457578 date "1983-01-01" @default.
- W243457578 modified "2023-09-27" @default.
- W243457578 title "Studies of initial reaction steps in the gasification of coal and selected model compounds. Final technical report, September 1981-August 1983" @default.
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