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• W2440665797 startingPage "20150139" @default.
• W2440665797 abstract "Cellulose nanocrystals (CNCs) are negatively charged colloidal particles well known to form highly stable surfactant-free Pickering emulsions. These particles can vary in surface charge density depending on their preparation by acid hydrolysis or applying post-treatments. CNCs with three different surface charge densities were prepared corresponding to 0.08, 0.16 and 0.64 e nm −2 , respectively. Post-treatment might also increase the surface charge density. The well-known TEMPO-mediated oxidation substitutes C 6 -hydroxyl groups by C 6 -carboxyl groups on the surface. We report that these different modified CNCs lead to stable oil-in-water emulsions. TEMPO-oxidized CNC might be the basis of further modifications. It is shown that they can, for example, lead to hydrophobic CNCs with a simple method using quaternary ammonium salts that allow producing inverse water-in-oil emulsions. Different from CNC modification before emulsification, modification can be carried out on the droplets after emulsification. This way allows preparing functional capsules according to the layer-by-layer process. As a result, it is demonstrated here the large range of use of these biobased rod-like nanoparticles, extending therefore their potential use to highly sophisticated formulations. This article is part of the themed issue ‘Soft interfacial materials: from fundamentals to formulation’." @default.
• W2440665797 created "2016-06-24" @default.
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• W2440665797 date "2016-07-28" @default.
• W2440665797 modified "2023-10-17" @default.
• W2440665797 title "Some modification of cellulose nanocrystals for functional Pickering emulsions" @default.
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• W2440665797 doi "https://doi.org/10.1098/rsta.2015.0139" @default.
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