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• W2444238538 abstract "The initial application is reported of single-crystal 55Mn NMR spectroscopy, and associated orientation dependence studies, to single-molecule magnets (SMMs). The studies were performed on two members of the Mn12 family of SMMs, [Mn12O12(O2CMe)16(H2O)4]·2MeCO2H·4H2O (Mn12−Ac) and [Mn12O12(O2CCH2Br)16(H2O)4]·4CH2Cl2 (Mn12−BrAc). Single-crystal spectra give a dramatic improvement in the spectral resolution over oriented powder spectra, allowing the clear observation of quadrupolar splittings, the determination of quadrupole coupling parameters (e2qQ), and an assessment of the symmetry-lowering perturbation of the core of Mn12−Ac by hydrogen-bonding interactions with lattice solvate molecules of crystallization. The results emphasize the utility of single-crystal NMR studies to probe the cores of these magnetic molecules." @default.
• W2444238538 created "2016-06-24" @default.
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• W2444238538 date "2005-03-01" @default.
• W2444238538 modified "2023-09-23" @default.
• W2444238538 title "Single-Crystal ⁵⁵Mn NMR Spectra of Two Mn₁₂ Single-Molecule Magnets" @default.
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• W2444238538 doi "https://doi.org/10.1021/ic050048j" @default.
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